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Active dipole clusters: from helical motion to fission

机译:有源偶极子团:从螺旋运动到裂变

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摘要

The structure of a finite particle cluster is typically determined by totalenergy minimization. Here we consider the case where a cluster of soft spheredipoles becomes active, i.e. when the individual particles exhibit anadditional self-propulsion along their dipole moments. We numerically solve theoverdamped equations of motion for soft-sphere dipoles in a solvent. Startingfrom an initial metastable dipolar cluster, the self-propulsion generates acomplex cluster dynamics. The final cluster state has in general a structurewidely different to the initial one, the details depend on the model parametersand on the protocol of how the self-propulsion is turned on. The center-of-massof the cluster moves on a helical path, the details of which are governed bythe initial cluster magnetization. An instantaneous switch to a highself-propulsion leads to fission of the cluster. However, fission does notoccur if the self-propulsion is increased slowly to high strengths. Ourpredictions can be verified through experiments with self-phoretic colloidalJanus-particles and for macroscopic self-propelled dipoles in a highly viscoussolvent.
机译:有限粒子簇的结构通常由总能量最小化确定。在这里,我们考虑一种情况,其中一簇软的球形偶极子变得活跃,即当单个粒子沿其偶极矩表现出附加的自推进力时。我们用数值方法求解了溶剂中软球偶极子的过阻尼运动方程。从初始的亚稳态偶极星团开始,自推进会产生复杂的星团动力学。最终的星团状态通常在结构上与初始的星团状态大不相同,其细节取决于模型参数以及如何开启自推进的协议。团簇的质心沿螺旋路径运动,其细节由初始团簇磁化强度控制。瞬间切换到高自我推进力会导致星团裂变。但是,如果将自我推进缓慢提高到高强度,则不会发生裂变。我们的预测可以通过在自粘性胶体Janus粒子上进行实验以及在高粘度溶剂中用于宏观自推进偶极子的实验来验证。

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